Inverse Materials Design

Solid-state physics ยท first-principles calculations ยท inverse design

Inverse Materials Design

We connect atomic-scale theory with target functionality, using density functional theory, descriptors, and data-driven workflows to identify which materials and configurations are worth synthesizing before expensive trial-and-error begins.

Atomic mechanisms DFT-based insight into structure, defects, and interfaces.
Targeted discovery Inverse design rules for materials with desired functions.
Useful workflows Open, reproducible analysis for real materials questions.

Scientific vision

Design from mechanism, not guesswork

The group develops physical insight and practical computational workflows for solid-state materials where structure, defects, disorder, and interfaces define performance.

Target a function

Start with desired electrochemical, electronic, or interfacial behavior rather than a fixed composition.

Resolve the real structure

Account for local symmetry breaking, polymorphous configurations, defects, disorder, and active interfaces.

Build descriptors

Turn first-principles data into interpretable relationships between atomic structure and target properties.

Guide synthesis

Prioritize candidates and conditions that have a credible path to experimental realization.

Research focus

Atomic insight for materials that must actually work

Current directions include energy-storage materials, intrinsic defects and doping, polymorphous compounds, and gapped-metal systems where small structural changes have large consequences.

Energy storage Hard carbon, polymer electrolytes, ion transport, plateau capacity, and interface stability.
Defects and doping Intrinsic defects, antidoping, non-stoichiometry, and property control in real compounds.
Polymorphous materials Local symmetry breaking in materials that appear high-symmetry in averaged measurements.
Gapped metals Electronic structure, dielectric response, and Casimir-Lifshitz behavior in unusual conductors.

Recent papers

Selected 2026 work

PRX Energy 2026 Carbon anodes

Rational design principles for Na- and Li-ion carbon anodes from interlayer spacing control

I. Radchenko, O. I. Malyi*

Defines practical interlayer-spacing targets for Li and Na storage in carbon anodes using first-principles and cluster-expansion modeling.

Corresponding author: O. I. Malyi

DOI: 10.1103/g52s-znhz
Graphical abstract for lattice reconstruction hard carbon paper
EES 2026 Fast charging

Lattice reconstruction strategy for fast-charging plateau-type hard carbon anode

F. Wang, L. Chen, F. Li, Y. Zheng, J. Wei, C. Diao, I. Radchenko, S. Jie, L. Li, J. Wang, Z. Bai, Y. Zhang, O. I. Malyi*, X. Chen, Y. Tang*

A hard-carbon reconstruction route balances interlayer distance, crystallite width, and interface chemistry for ultra-long-life sodium-ion batteries.

Corresponding authors: O. I. Malyi, Y. Tang

DOI: 10.1039/D6EE00708B
Graphical abstract for polyamine mediated solid polymer electrolyte paper
Advanced Materials 2026 Solid-state batteries

Polyamine-mediated proton/TFSI- dual capture enables high-voltage PEO-based all-solid-state Li batteries

Y. Fan, M. Zhu, H. Wang, Z. Hong, B. Zhao, H. Ke, Y. Jiang, M. Zhu, P. Chen, Z. Liu, Z. Bai, S. Chen, H. Shao, O. I. Malyi*, Y. Tang*

A stabilization strategy suppresses acid-catalyzed PEO degradation and improves high-voltage all-solid-state lithium battery cycling.

Corresponding authors: O. I. Malyi, Y. Tang

DOI: 10.1002/adma.202520538

Latest news

Dr. Gabriel Kuderowicz
May 2026 ยท New group member

Welcome Dr. Gabriel Kuderowicz

Dr. Gabriel Kuderowicz joins Ensemble3 as a postdoctoral researcher focused on hard carbon materials for sodium-ion batteries.

Role: Postdoc, Ensemble3, Poland, May 2026 -

April 2026 ยท Publication

Hard-carbon lattice reconstruction paper published in Energy & Environmental Science

The study reports a fast-charging plateau-type hard carbon anode with long cycle life by tuning graphitic domains and solid-electrolyte interphase chemistry.

Corresponding authors: O. I. Malyi, Y. Tang

DOI: 10.1039/D6EE00708B
April 2026 ยท Publication

Rational design principles for Na- and Li-ion carbon anodes

The work establishes spacing-dependent design rules for alkali-metal intercalation in expanded graphite and hard-carbon-relevant domains.

Corresponding author: O. I. Malyi

DOI: 10.1103/g52s-znhz
January 2026 ยท Publication

Polyamine-mediated proton/TFSI- dual capture for high-voltage PEO-based ASSLBs

Corresponding authors: O. I. Malyi, Y. Tang. Advanced Materials, 2026.

View paper
October 2025 ยท Publication

Lewis-acid fluorides for high-performance solid-state polymer electrolytes

Corresponding authors: O. I. Malyi, Y. Tang. Science China Materials, 2026.

View paper
November 2025 ยท New group member

Welcome Dr. Andrรฉs Felipe Usuga

Dr. Andrรฉs Felipe Usuga joined Ensemble3 as a postdoctoral researcher focused on hard carbon materials for sodium-ion batteries.

Members
October 2025 ยท Publication

Breaking diffusion limit in ester-flame-proof Na-ion electrolytes

Corresponding authors: Y. Zhang, O. I. Malyi, Y. Tang. Angewandte Chemie, 2025.

View paper
February 2025 ยท Publication

Pushing slope- to plateau-type behavior in hard carbon for sodium-ion batteries

Corresponding authors: O. I. Malyi, Y. Tang, X. Bao. Energy & Environmental Science, 2025.

View paper
February 2025 ยท Publication

Surface-confined disordered hydrogen bonds enable efficient lithium transport

Y. Fan, O. I. Malyi, H. Wang et al. Angewandte Chemie, 2025. Equal contribution; hot paper.

View paper
March 2025 ยท Publication

Unveiling defect physics in gapped metals

Corresponding author: O. I. Malyi. Journal of Materials Informatics, 2025.

View paper
February 2025 ยท Publication

Mechanism for ice growth on the surface of a spherical water droplet

Y. Li, P. Parashar, T. Jayasekera, I. Brevik, C. Persson, O. I. Malyi, M. Bostrรถm. Physical Review B, 2025.

View paper
February 2025 ยท Publication

Impact of metal oxidation on growth and melting of ice

S. Carretero-Palacios, V. Esteso, Y. Li, S. Kuthe, I. Brevik, K. Iordanidou, O. I. Malyi et al. Physical Review B, 2025.

View paper
January 2025 ยท Publication

Beyond attraction: controllable off-stoichiometry in gapped metals

S. Pal, S. Osella, O. I. Malyi, M. Bostrรถm. Physics Letters A, 2025.

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Full publication list

See the complete publication record and representative works.

All publications

Join us

Open to strong candidates in computational materials discovery

The group welcomes researchers who are excited by solid-state physics, first-principles calculations, data-driven materials design, and the challenge of turning atomic-scale mechanisms into design rules.

Fellowship-minded candidates are very welcome. Strong postdoctoral applicants can contact the group to discuss project ideas and potential host support for routes such as Marie Skล‚odowska-Curie Actions Postdoctoral Fellowships, the NAWA Ulam Programme, and similar international fellowship schemes.

MSCA PF NAWA Ulam International fellowships